Two men are due in court on Wednesday and a third has been charged in what police allege was the organised theft of more than 75 bikes in inner Sydney.

Officers from Redfern Police Area Command began investigating the thefts at the beginning of the year, after bikes were stolen from inner city suburbs including Alexandria.

Police said most of the bikes were stolen from bike storage cages, such as this one, inside residential buildings. Credit:Fairfax Media

Police said the bicycles, including two worth more than $6000 each, were mostly stolen from bike cages inside residential car parks.

On Tuesday, officers searched a home on Darling Avenue in Lurnea, near Liverpool, and arrested three men. Police also seized three bicycles and three motorbikes.