Metamaterials provide a powerful platform to probe and enhance nonlinear responses in physical systems toward myriad applications. Herein, the development of a coupled nonlinear metamaterial (NLMM) featuring a self‐adaptive response that selectively amplifies the magnetic field is reported. The resonance of the NLMM is suppressed in response to higher degrees of radio‐frequency excitation strength and recovers during a subsequent low excitation strength phase, thereby exhibiting an intelligent, or nonlinear, behavior by passively sensing excitation signal strength and responding accordingly. The nonlinear response of the NLMM enables us to boost the signal‐to‐noise ratio during magnetic resonance imaging to an unprecedented degree. These results provide insights into a new paradigm to construct NLMMs consisting of coupled resonators and pave the way toward the utilization of NLMMs to address a host of practical technological applications.